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11,11,12,12-Tetracyanonaphtho-2,6-quinodimethane in contact with ferromagnetic electrodes for organic spintronics
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Shi, Shengwei, Sun, Zhengyi, Liu, Xianjie, Bedoya-Pinto, Amilcar, Graziosi, Patrizio, Yu, Huangzhong, Li, Wenting, Liu, Gang, Hueso, Luis, Dediu, Valentin A. and Fahlman, Mats (2018) 11,11,12,12-Tetracyanonaphtho-2,6-quinodimethane in contact with ferromagnetic electrodes for organic spintronics. Advanced Electronic Materials , 4 (7). 1800077. doi:10.1002/aelm.201800077 ISSN 2199-160X.
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Official URL: http://dx.doi.org/10.1002/aelm.201800077
Abstract
Spinterface engineering has shown quite important roles in organic spintronics as it can improve spin injection or extraction. In this study, 11,11,12,12‐tetracyanonaptho‐2,6‐quinodimethane (TNAP) is introduced as an interfacial layer for a prototype interface of Fe/TNAP. An element‐specific investigation of the electronic and magnetic structures of Fe/TNAP system by use of near edge X‐Ray absorption fine structure (NEXAFS) and X‐ray magnetic circular dichroism (XMCD) is reported. Strong hybridization between TNAP and Fe and induced magnetization of N atoms in TNAP molecule are observed. XMCD sum rule analysis demonstrates that the adsorption of TNAP reduces the spin moment of Fe by 12%. In addition, induced magnetization in N K‐edge of TNAP is also found with other commonly used ferromagnets in organic spintronics, such as La0.7Sr0.3MnO3 and permalloy, which makes TNAP a very promising molecule for spinterface engineering in organic spintronics.
Item Type: | Journal Article | ||||||||
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Divisions: | Faculty of Science, Engineering and Medicine > Engineering > Engineering | ||||||||
Journal or Publication Title: | Advanced Electronic Materials | ||||||||
Publisher: | Wiley-Blackwell Publishing Ltd. | ||||||||
ISSN: | 2199-160X | ||||||||
Official Date: | July 2018 | ||||||||
Dates: |
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Volume: | 4 | ||||||||
Number: | 7 | ||||||||
Article Number: | 1800077 | ||||||||
DOI: | 10.1002/aelm.201800077 | ||||||||
Status: | Peer Reviewed | ||||||||
Publication Status: | Published | ||||||||
Access rights to Published version: | Restricted or Subscription Access |
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