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Thermodynamic discontinuity between low-density amorphous ice and supercooled water
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UNSPECIFIED (2002) Thermodynamic discontinuity between low-density amorphous ice and supercooled water. PHYSICAL REVIEW LETTERS, 88 (15). -. doi:10.1103/PhysRevLett.88.155502 ISSN 0031-9007.
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Official URL: http://dx.doi.org/10.1103/PhysRevLett.88.155502
Abstract
A combination of reverse Monte Carlo, molecular dynamics, and lattice dynamics simulations were used to obtain structural and thermodynamic data for low-density amorphous ice. A thermodynamically discontinuous transformation to a phase with properties and a structure consistent with supercooled liquid water is found to occur at similar to130 K . Quantum corrections have a profound effect on thermodynamic properties and the location of important thermodynamic points in the water phase diagram.
| Item Type: | Journal Article | ||||
|---|---|---|---|---|---|
| Subjects: | Q Science > QC Physics | ||||
| Journal or Publication Title: | PHYSICAL REVIEW LETTERS | ||||
| Publisher: | AMERICAN PHYSICAL SOC | ||||
| ISSN: | 0031-9007 | ||||
| Official Date: | 15 April 2002 | ||||
| Dates: |
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| Volume: | 88 | ||||
| Number: | 15 | ||||
| Number of Pages: | 4 | ||||
| Page Range: | - | ||||
| DOI: | 10.1103/PhysRevLett.88.155502 | ||||
| Publication Status: | Published |
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