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Hierarchical nanostructuring approaches for thermoelectric materials with high power factors
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Vargiamidis, Vassilios and Neophytou, Neophytos (2019) Hierarchical nanostructuring approaches for thermoelectric materials with high power factors. Physical Review B (Condensed Matter and Materials Physics), 99 (4). 045405 . doi:10.1103/PhysRevB.99.045405 ISSN 1098-0121.
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WRAP-hierarchical-nanostructuring-approaches-TE-Neophytou-2019.pdf - Accepted Version - Requires a PDF viewer. Download (2053Kb) | Preview |
Official URL: http://dx.doi.org/10.1103/PhysRevB.99.045405
Abstract
The thermoelectric power factor of hierarchically nanostructured materials is investigated using the nonequilibrium Green's function method for quantum transport, including interactions of electrons with acoustic and optical phonons. We describe hierarchical nanostructuring by superlattice-like potential barriers/wells, combined with quantum dot barriers/wells nanoinclusions as well as voids in the intermediate region. We show that these structures can be designed in a way that the power factor is not only largely immune to the presence of the nanostructure features, but under certain conditions benefits can be achieved as well. Interestingly, we show that these design approaches are linked to the energy relaxation of the current flow and whether charge carrier scattering is limited by elastic or inelastic processes. In particular, when nanostructures form potential barriers, the power factor can be substantially enhanced under elastic scattering conditions, irrespective of nanostructuring density and potential barrier heights. When inelastic scattering processes dominate, however, the power factor is inevitably degraded. In the case in which nanostructures form potential wells, despite a slight decrease, the power factor is quite resilient under either elastic or inelastic scattering processes. These nanostructuring design approaches could help open the path to the optimization of new generation nanostructured thermoelectric materials by not only targeting reductions in thermal conductivity, but simultaneous improvements in the power factor as well.
| Item Type: | Journal Article | ||||||
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| Subjects: | Q Science > QC Physics T Technology > TA Engineering (General). Civil engineering (General) T Technology > TK Electrical engineering. Electronics Nuclear engineering |
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| Divisions: | Faculty of Science, Engineering and Medicine > Engineering > Engineering | ||||||
| Library of Congress Subject Headings (LCSH): | Nanostructured materials, Superlattices as materials, Thermoelectric materials | ||||||
| Journal or Publication Title: | Physical Review B (Condensed Matter and Materials Physics) | ||||||
| Publisher: | American Physical Society | ||||||
| ISSN: | 1098-0121 | ||||||
| Official Date: | 7 January 2019 | ||||||
| Dates: |
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| Volume: | 99 | ||||||
| Number: | 4 | ||||||
| Article Number: | 045405 | ||||||
| DOI: | 10.1103/PhysRevB.99.045405 | ||||||
| Status: | Peer Reviewed | ||||||
| Publication Status: | Published | ||||||
| Reuse Statement (publisher, data, author rights): | © 2019 American Physical Society | ||||||
| Access rights to Published version: | Restricted or Subscription Access | ||||||
| Date of first compliant deposit: | 15 January 2019 | ||||||
| Date of first compliant Open Access: | 16 January 2019 | ||||||
| RIOXX Funder/Project Grant: |
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