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Consolidated production of coniferol and other high-value aromatic alcohols directly from lignocellulosic biomass
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Tramontina, Robson, Galman, James L., Parmeggiani, Fabio, Derrington, Sasha R., Bugg, Timothy D. H., Turner, Nicholas J., Squina, Fabio M. and Dixon, Neil (2020) Consolidated production of coniferol and other high-value aromatic alcohols directly from lignocellulosic biomass. Green Chemistry, 22 (1). pp. 144-152. doi:10.1039/c9gc02359c
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WRAP-consolidated-production-coniferol-high-value-alchols-Bugg-2020.pdf - Published Version - Requires a PDF viewer. Available under License Creative Commons Attribution. Download (2117Kb) | Preview |
Official URL: http://dx.doi.org/10.1039/c9gc02359c
Abstract
Sustainable production of fine chemicals and biofuels from renewable biomass offers a potential alternative to the continued use of finite geological oil reserves. However, in order to compete with current petrochemical refinery processes, alternative biorefinery processes must overcome significant costs and productivity barriers. Herein, we demonstrate the biocatalytic production of the versatile chemical building block, coniferol, for the first time, directly from lignocellulosic biomass. Following the biocatalytic treatment of lignocellulose to release and convert ferulic acid with feruloyl esterase (XynZ), carboxylic acid reductase (CAR) and aldo-keto reductase (AKR), this whole cell catalytic cascade not only achieved equivalent release of ferulic acid from lignocellulose compared to alkaline hydrolysis, but also displayed efficient conversion of ferulic acid to coniferol. This system represents a consolidated biodegradation–biotransformation strategy for the production of high value fine chemicals from waste plant biomass, offering the potential to minimize environmental waste and add value to agro-industrial residues.
| Item Type: | Journal Article | ||||||||||||||||||
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| Subjects: | Q Science > QD Chemistry T Technology > TP Chemical technology |
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| Divisions: | Faculty of Science > Chemistry | ||||||||||||||||||
| SWORD Depositor: | Library Publications Router | ||||||||||||||||||
| Library of Congress Subject Headings (LCSH): | Carboxylic acids, Lignocellulose, Plant biomass , Environmental chemistry | ||||||||||||||||||
| Journal or Publication Title: | Green Chemistry | ||||||||||||||||||
| Publisher: | Royal Society of Chemistry (RSC) | ||||||||||||||||||
| ISSN: | 1463-9270 | ||||||||||||||||||
| Official Date: | January 2020 | ||||||||||||||||||
| Dates: |
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| Volume: | 22 | ||||||||||||||||||
| Number: | 1 | ||||||||||||||||||
| Page Range: | pp. 144-152 | ||||||||||||||||||
| DOI: | 10.1039/c9gc02359c | ||||||||||||||||||
| Status: | Peer Reviewed | ||||||||||||||||||
| Publication Status: | Published | ||||||||||||||||||
| Publisher Statement: | ** Article version: VoR ** From Crossref via Jisc Publications Router ** Licence for VoR version of this article starting on 25-11-2019: http://creativecommons.org/licenses/by/3.0/ | ||||||||||||||||||
| Access rights to Published version: | Open Access | ||||||||||||||||||
| RIOXX Funder/Project Grant: |
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