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Ashfold, Michael N. R., Goss, Jonathan P., Green, Ben L., May, Paul W., Newton, Mark E. and Peaker, Chloe V. (2020) Nitrogen in diamond. Chemical Reviews, 12 . pp. 5745-5794. doi:10.1021/acs.chemrev.9b00518 ISSN 0009-2665.
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Official URL: http://dx.doi.org/10.1021/acs.chemrev.9b00518
Abstract
Nitrogen is ubiquitous in both natural and laboratory-grown diamond, but the number and nature of the nitrogen-containing defects can have a profound effect on the diamond material and its properties. An ever-growing fraction of the supply of diamond appearing on the world market is now lab-grown. Here, we survey recent progress in two complementary diamond synthesis methods—high pressure high temperature (HPHT) growth and chemical vapor deposition (CVD), how each is allowing ever more precise control of nitrogen incorporation in the resulting diamond, and how the diamond produced by either method can be further processed (e.g., by implantation or annealing) to achieve a particular outcome or property. The burgeoning availability of diamond samples grown under well-defined conditions has also enabled huge advances in the characterization and understanding of nitrogen-containing defects in diamond—alone and in association with vacancies, hydrogen, and transition metal atoms. Among these, the negatively charged nitrogen-vacancy (NV–) defect in diamond is attracting particular current interest in account of the many new and exciting opportunities it offers for, for example, quantum technologies, nanoscale magnetometry, and biosensing.
| Item Type: | Journal Article | |||||||||||||||
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| Subjects: | Q Science > QE Geology T Technology > TJ Mechanical engineering and machinery |
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| Divisions: | Faculty of Science, Engineering and Medicine > Science > Physics | |||||||||||||||
| Library of Congress Subject Headings (LCSH): | Diamonds , Diamonds, Industrial , Diamonds -- Nitrogen content | |||||||||||||||
| Journal or Publication Title: | Chemical Reviews | |||||||||||||||
| Publisher: | American Chemical Society | |||||||||||||||
| ISSN: | 0009-2665 | |||||||||||||||
| Official Date: | 24 June 2020 | |||||||||||||||
| Dates: |
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| Volume: | 12 | |||||||||||||||
| Page Range: | pp. 5745-5794 | |||||||||||||||
| DOI: | 10.1021/acs.chemrev.9b00518 | |||||||||||||||
| Status: | Peer Reviewed | |||||||||||||||
| Publication Status: | Published | |||||||||||||||
| Reuse Statement (publisher, data, author rights): | This document is the Accepted Manuscript version of a Published Work that appeared in final form in Chemical Reviews, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see http://dx.doi.org/10.1021/acs.chemrev.9b00518 | |||||||||||||||
| Access rights to Published version: | Restricted or Subscription Access | |||||||||||||||
| Date of first compliant deposit: | 4 March 2020 | |||||||||||||||
| Date of first compliant Open Access: | 12 February 2021 | |||||||||||||||
| RIOXX Funder/Project Grant: |
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