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A study on the influence of lithium plating on battery degradation

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Koleti, Upender Rao, Rajan, Ashwin T., Tan, Chaou C., Moharana, Sanghamitra, Dinh, Truong Quang and Marco, James (2020) A study on the influence of lithium plating on battery degradation. Energies, 13 (13). 3458. doi:10.3390/en13133458 ISSN 1996-1073.

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Official URL: http://dx.doi.org/10.3390/en13133458

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Abstract

Within Li-ion batteries, lithium plating is considered as one of the main reasons behind the capacity fade that occurs during low temperature and fast charging conditions. Previous studies indicate that plating is influenced by the levels of loss of lithium inventory (LLI) and the loss of active material (LAM) present in a battery. However, it is not clear from the literature on how lithium plating influences battery degradation in terms of LAM and LLI. Quantifying the undesirable impacts of lithium plating can help in understanding its impact on battery degradation and feedback effects of previous lithium plating on the formation of present plating. This study aims to quantify the degradation modes of lithium plating: LLI, LAM at the electrode level. A commercial Li-ion cell was first, aged using two different cases: with and without lithium plating. Second, a degradation diagnostic method is developed to quantify the degradation modes based on their measurable effects on open-circuit voltage (OCV) and cell capacity. The results highlight that LAMNE and LLI levels under the fast charge profile are increased by 10% and 12%, respectively, compared to those under the less aggressive charge profile. Further, limitations of the degradation analysis methods are discussed.

Item Type: Journal Article
Subjects: T Technology > TA Engineering (General). Civil engineering (General)
T Technology > TJ Mechanical engineering and machinery
T Technology > TK Electrical engineering. Electronics Nuclear engineering
T Technology > TS Manufactures
Divisions: Faculty of Science, Engineering and Medicine > Engineering > WMG (Formerly the Warwick Manufacturing Group)
Library of Congress Subject Headings (LCSH): Lithium ion batteries, Lithium ion batteries -- Materials, Battery management systems, Plating, Lithium
Journal or Publication Title: Energies
Publisher: M.D.P.I.A.G.
ISSN: 1996-1073
Official Date: 3 July 2020
Dates:
DateEvent
3 July 2020Published
26 June 2020Accepted
Volume: 13
Number: 13
Article Number: 3458
DOI: 10.3390/en13133458
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Open Access (Creative Commons)
Date of first compliant deposit: 9 July 2020
Date of first compliant Open Access: 15 July 2020

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