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Brønsted acid-based strategies for N-heterocyclic synthesis
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Henry, Stuart Adam (2019) Brønsted acid-based strategies for N-heterocyclic synthesis. PhD thesis, University of Warwick.
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Official URL: http://webcat.warwick.ac.uk/record=b3493261~S15
Abstract
The focal point of this work has been the development of new and expedient Brønsted acid–catalysed synthetic methods with alcohol pro–electrophiles to rapidly achieve molecular complexity.
Chapter 1 provides insight into notable developments within the field of Brønsted acid–mediated transformations of alcohols as pro–electrophiles.
Chapter 2 describes our efforts towards the realisation of a chiral Brønsted acid– catalysed enantioselective 1,3–allylic alcohol isomerisation of 3–indolinols.
Chapter 3 describes the synthesis of 1,2–dihydroquinolines via a Brønsted acid–catalysed intramolecular allylic amination.
Chapter 4 is an account of the Brønsted acid–catalysed cyclisation of b–amino–1,4– enols to oxazol–2(3H)–ones and 5–alkenyloxazolidin–2–ones.
Chapter 5 provides a summary of the works presented herein.
Chapter 6 details the experimental data and methods used in the work presented in this thesis.
Item Type: | Thesis or Dissertation (PhD) | ||||
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Subjects: | Q Science > QD Chemistry | ||||
Library of Congress Subject Headings (LCSH): | Heterocyclic compounds -- Synthesis, Catalysis, Electrophiles | ||||
Official Date: | August 2019 | ||||
Dates: |
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Institution: | University of Warwick | ||||
Theses Department: | Department of Chemistry | ||||
Thesis Type: | PhD | ||||
Publication Status: | Unpublished | ||||
Supervisor(s)/Advisor: | Chan, Philip Wai Hong | ||||
Sponsors: | Engineering and Physical Sciences Research Council ; University of Warwick | ||||
Format of File: | |||||
Extent: | vii, 198 leaves : illustrations (some colour) | ||||
Language: | eng |
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