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Magnetic structure and low-temperature properties of geometrically frustrated SrNd2O4

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Qureshi, N., Wildes, A. R., Ritter, C., Fåk, B., Riberolles, S. X. M., Ciomaga Hatnean, Monica and Petrenko, Oleg (2021) Magnetic structure and low-temperature properties of geometrically frustrated SrNd2O4. Physical Review B, 103 (13). 134433. doi:10.1103/PhysRevB.103.134433 ISSN 2469-9950.

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Official URL: http://dx.doi.org/10.1103/PhysRevB.103.134433

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Abstract

We report the low-temperature properties of SrNd2O4, a geometrically frustrated magnet. Magnetization and heat capacity measurements performed on polycrystalline samples indicate the appearance of a magnetically ordered state at TN = 2.28(4)K. Powder neutron diffraction measurements reveal that an antiferromagnetic state with the propagation vector q = (0 1/2 1/2 ) is stabilized below this temperature. The magnetic order is incomplete, as only one of the two Nd3+ sites carries a significant magnetic moment while the other site remains largely disordered. The presence of a disordered magnetic component below TN is confirmed with polarized neutron diffraction measurements. In an applied magnetic field, the bulk property measurements indicate a phase transition at about 30 kOe. We construct a tentative H-T phase diagram of SrNd2O4 from these measurements.

Item Type: Journal Article
Subjects: Q Science > QC Physics
Divisions: Faculty of Science, Engineering and Medicine > Science > Physics
Library of Congress Subject Headings (LCSH): Rare earth metals -- Magnetic properties, Strontium compounds -- Magnetic properties, Neutrons -- Diffraction, Neutrons -- Inelastic scattering
Journal or Publication Title: Physical Review B
Publisher: American Physical Society
ISSN: 2469-9950
Official Date: 1 April 2021
Dates:
DateEvent
1 April 2021Published
22 April 2021Available
6 April 2021Accepted
14 December 2020Submitted
Volume: 103
Number: 13
Article Number: 134433
DOI: 10.1103/PhysRevB.103.134433
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access
Copyright Holders: ©2021 American Physical Society
Date of first compliant deposit: 23 April 2021
Date of first compliant Open Access: 26 April 2021
RIOXX Funder/Project Grant:
Project/Grant IDRIOXX Funder NameFunder ID
EP/T005963/1[EPSRC] Engineering and Physical Sciences Research Councilhttp://dx.doi.org/10.13039/501100000266

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