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Manganese-catalyzed batch and continuous flow cationic RAFT polymerization induced by visible light
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Li, Jiajia, Kerr, Andrew, Song, Qiao, Yang, Jie, Häkkinen, Satu, Pan, Xiangqiang, Zhang, Zhengbiao, Zhu, Jian and Perrier, Sébastien (2021) Manganese-catalyzed batch and continuous flow cationic RAFT polymerization induced by visible light. ACS Macro Letters, 10 . pp. 570-575. doi:10.1021/acsmacrolett.1c00180
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WRAP-manganese-catalyzed-batch-continuous-flow-cationic-RAFT-polymerization-induced-visible-light-Perrier-2021 .pdf - Accepted Version - Requires a PDF viewer. Download (1579Kb) | Preview |
Official URL: http://dx.doi.org/10.1021/acsmacrolett.1c00180
Abstract
We present a robust manganese-catalyzed cationic reversible addition–fragmentation chain transfer (RAFT) polymerization induced by visible light. Well-defined poly(vinyl ether)s with controlled molecular weight and molecular weight distributions (MWDs) can be conveniently prepared at room temperature without monomer purification. The commercially available manganese carbonyl bromide is used as the photocatalyst for cationic RAFT polymerization. Moreover, this method has been further applied in both batch and continuous flow systems, providing a visible light induced flow cationic polymerization under mild conditions.
| Item Type: | Journal Item | |||||||||
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| Subjects: | Q Science > QD Chemistry | |||||||||
| Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry | |||||||||
| Library of Congress Subject Headings (LCSH): | Manganese, Manganese catalysts , Addition polymerization | |||||||||
| Journal or Publication Title: | ACS Macro Letters | |||||||||
| Publisher: | American Chemical Society | |||||||||
| ISSN: | 2161-1653 | |||||||||
| Official Date: | 21 April 2021 | |||||||||
| Dates: |
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| Volume: | 10 | |||||||||
| Page Range: | pp. 570-575 | |||||||||
| DOI: | 10.1021/acsmacrolett.1c00180 | |||||||||
| Status: | Peer Reviewed | |||||||||
| Publication Status: | Published | |||||||||
| Reuse Statement (publisher, data, author rights): | This document is the Accepted Manuscript version of a Published Work that appeared in final form in ACS Macro Letters, copyright © American Chemical Society after peer review and technical editing by the publisher. To access the final edited and published work see http://dx.doi.org/10.1021/acsmacrolett.1c00180 | |||||||||
| Access rights to Published version: | Restricted or Subscription Access | |||||||||
| Date of first compliant deposit: | 23 April 2021 | |||||||||
| Date of first compliant Open Access: | 21 April 2022 | |||||||||
| RIOXX Funder/Project Grant: |
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