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Magnetic structure investigation of the intercalated transition metal dichalcogenide V1/3NbS2

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Hall, A. E., Khalyavin, D. D., Manuel, P., Mayoh, Daniel, Orlandi, F., Petrenko, Oleg, Lees, Martin R. and Balakrishnan, Geetha (2021) Magnetic structure investigation of the intercalated transition metal dichalcogenide V1/3NbS2. Physical Review B, 103 (17). 174431. doi:10.1103/PhysRevB.103.174431

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Official URL: http://dx.doi.org/10.1103/PhysRevB.103.174431

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Abstract

We investigate the temperature evolution of the magnetic structure of V1/3NbS2 using neutron diffraction techniques. We find that V1/3NbS2 has two propagation vectors: k0 = (0, 0, 0) and k1 = (0, 0, 1/3 ). The k0 vector can be associated with an antiferromagnetic ordering of in-plane moments with a refined value of 0.90(5)μB, and k1 can be associated with moments along the c axis in an up-down-down configuration with refined values of 1.21(12)μB and 0.61(6)μB. Both k0 and k1 magnetic components couple with an out-of-plane ferromagnetic moment consistent with magnetization data. Furthermore, single-crystal neutron diffraction shows evidence of diffuse magnetic scattering between the (010) and (01±1/3 ) Bragg peaks. We also characterize the field and temperature evolution of the magnetic structure in V1/3NbS2 by magnetic susceptibility and heat capacity measurements. The dc susceptibility measurements give an antiferromagnetic transition temperature of TN = 50 K, and the field scans reveal that the moment does not saturate at magnetic fields up to 100 kOe.

Item Type: Journal Article
Subjects: Q Science > QC Physics
Divisions: Faculty of Science > Physics
Library of Congress Subject Headings (LCSH): Neutrons -- Diffraction, Transition metals -- Magnetic properties, Antiferromagnetism
Journal or Publication Title: Physical Review B
Publisher: American Physical Society
ISSN: 2469-9950
Official Date: 1 May 2021
Dates:
DateEvent
1 May 2021Published
25 May 2021Available
3 May 2021Accepted
24 February 2021Submitted
Volume: 103
Number: 17
Article Number: 174431
DOI: 10.1103/PhysRevB.103.174431
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access
Copyright Holders: ©2021 American Physical Society
RIOXX Funder/Project Grant:
Project/Grant IDRIOXX Funder NameFunder ID
EP/N032128/1[EPSRC] Engineering and Physical Sciences Research Councilhttp://dx.doi.org/10.13039/501100000266
UNSPECIFIEDUK Research and Innovationhttp://dx.doi.org/10.13039/100014013
UNSPECIFIED[STFC] Science and Technology Facilities Councilhttp://dx.doi.org/10.13039/501100000271

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