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Magnetic anisotropy of individually addressed spin states
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Peters, L. C. J. M., Christianen, P. C. M., Engelkamp, H., Groenenboom, G. C., Maan, J. C., Kampert, Erik, Tinnemans, P. T., Rowan, A. E. and Zeitler, U. (2021) Magnetic anisotropy of individually addressed spin states. Physical Review Research, 3 (4). L042042 . doi:10.1103/PhysRevResearch.3.L042042
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WRAP-Magnetic-anisotropy-individually-addressed-spin-states-2021.pdf - Accepted Version - Requires a PDF viewer. Available under License Creative Commons Attribution 4.0. Download (1431Kb) | Preview |
Official URL: http://dx.doi.org/10.1103/PhysRevResearch.3.L04204...
Abstract
Controlling magnetic anisotropy is a key requirement for the fundamental understanding of molecular magnetism and is a prerequisite for numerous applications in magnetic storage, spintronics, and all-spin logic devices. In order to address the question of molecular magnetic anisotropy experimentally, we have synthesized single crystals of a molecular spin system containing four antiferromagnetically coupled s=5/2 manganese(II) ions. Using low-temperature cantilever magnetometry, we demonstrate the selective population of the
S=0,1,...,10 spin states upon application of magnetic fields up to 33 T and map the magnetic anisotropy of each of these states. We observe a strong dependence of the shape and size of the magnetic anisotropy on the populated spin states, and, in particular, reveal an anisotropy reversal upon going from the lowest to the highest spin state.
| Item Type: | Journal Article | ||||||||
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| Subjects: | Q Science > QC Physics Q Science > QD Chemistry T Technology > TK Electrical engineering. Electronics Nuclear engineering |
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| Divisions: | Faculty of Science, Engineering and Medicine > Engineering > WMG (Formerly the Warwick Manufacturing Group) | ||||||||
| Library of Congress Subject Headings (LCSH): | Anisotropy, Antiferromagnetism , Spintronics | ||||||||
| Journal or Publication Title: | Physical Review Research | ||||||||
| Publisher: | American Physical Society | ||||||||
| ISSN: | 2643-1564 | ||||||||
| Official Date: | 16 December 2021 | ||||||||
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| Volume: | 3 | ||||||||
| Number: | 4 | ||||||||
| Article Number: | L042042 | ||||||||
| DOI: | 10.1103/PhysRevResearch.3.L042042 | ||||||||
| Status: | Peer Reviewed | ||||||||
| Publication Status: | Published | ||||||||
| Access rights to Published version: | Open Access | ||||||||
| RIOXX Funder/Project Grant: |
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