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Effect of polymer molecular mass and structure on the mechanical properties of polymer–glass hybrids
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Lee, Yu Lin, Lester, Daniel, Jones, Julian R. and Georgiou, Theoni K. (2022) Effect of polymer molecular mass and structure on the mechanical properties of polymer–glass hybrids. ACS Omega, 7 (1). pp. 786-792. doi:10.1021/acsomega.1c05424 ISSN 2470-1343.
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WRAP-Effect-polymer-molecular-mass-structure-mechanical-2022.pdf - Published Version - Requires a PDF viewer. Available under License Creative Commons Attribution Non-commercial No Derivatives 4.0. Download (2422Kb) | Preview |
Official URL: https://doi.org/10.1021/acsomega.1c05424
Abstract
Organic–inorganic hybrid materials are a promising class of materials for tissue engineering and other biomedical applications. In this systematic study, the effect of the polymer molecular mass (MM) with a linear architecture on hybrid mechanical properties is reported. Well-defined linear poly(methyl methacrylate-co-(3-(trimethoxysilyl)propyl methacrylate)) polymers with a range of MMs of 9 to 90 kDa and one 90 kDa star-shaped polymer were synthesized and then used to form glass–polymer hybrids. It was demonstrated that increasing linear polymer MM decreases the resultant hybrid mechanical strength. Furthermore, a star-polymer hybrid was synthesized as a comparison and demonstrated significantly different mechanical properties relative to its linear-polymer counterpart.
| Item Type: | Journal Article | ||||||||
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| Subjects: | Q Science > QD Chemistry R Medicine > R Medicine (General) R Medicine > RC Internal medicine T Technology > TP Chemical technology |
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| Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry | ||||||||
| SWORD Depositor: | Library Publications Router | ||||||||
| Library of Congress Subject Headings (LCSH): | Bone regeneration, Tissue engineering -- Materials, Biomimetic polymers | ||||||||
| Journal or Publication Title: | ACS Omega | ||||||||
| Publisher: | American Chemical Society (ACS) | ||||||||
| ISSN: | 2470-1343 | ||||||||
| Official Date: | 11 January 2022 | ||||||||
| Dates: |
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| Volume: | 7 | ||||||||
| Number: | 1 | ||||||||
| Page Range: | pp. 786-792 | ||||||||
| DOI: | 10.1021/acsomega.1c05424 | ||||||||
| Status: | Peer Reviewed | ||||||||
| Publication Status: | Published | ||||||||
| Reuse Statement (publisher, data, author rights): | ** Article version: VoR ** From Crossref journal articles via Jisc Publications Router ** History: epub 22-12-2021; issued 22-12-2021. ** Licence for VoR version of this article starting on 22-12-2021: https://creativecommons.org/licenses/by-nc-nd/4.0/ | ||||||||
| Access rights to Published version: | Open Access (Creative Commons) | ||||||||
| Date of first compliant deposit: | 8 February 2022 | ||||||||
| Date of first compliant Open Access: | 8 February 2022 | ||||||||
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