The data have been collected in a single folder in the following order:


PMLG optimization:
===================

Record 304: tau_LG_expt vs 1H nutation frequency (1H 1D CRAMPS)  - Section 3.3, Figure 3 / Figure S1 / Figure S2

Record 305: tau_LG_expt vs tau_tilt (1H 1D CRAMPS) -  Section S3, Figure S3

Record 892-901: 1H spin-echo dephasing time (windowless PMLG5 - windowed PMLG9 - windowless PMLG9 - no 1H homonuclear decoupling - windowed PMLG5) - Section 3.4, Figure 4


1H 1D GHz data:
===================

Record 301: One-pulse 1H 1D  - Section 3.3, Figure 3

Record 302: 1H 1D CRAMPS (108 kHz)  - Section 3.3, Figure 3

Record 303: 1H 1D CRAMPS (51 kHz)  - Section 3.3, Figure 3


2D 1H-1H correlation:
===================

Record 306: no 1H homonuclear decoupling -  Section S4, Figure S4

Record 307: windowless PMLG9 - Section S4, Figure S4

Record 308: windowless PMLG5 -  Section S4, Figure S4


15N-1H CP- Refocused INEPT experiment:
================

Record 333: 2D 15N-1H CP- Refocused INEPT experiment (NA Glycine - Windowless PMLG9) - Section 3.1, Figure 1

Record 152-211: Frequency offset Windowed PMLG5  - Section 3.5, Figure 5 / Figure 7

Record 10-51: Frequency offset Windowed PMLG9 - Section 3.5, Figure S5 / Figure 7

Record 60-71: Frequency offset Windowless PMLG9 - Section 3.5, Figure S5 / Figure 7

Record 120-132: Frequency offset Windowless PMLG5 - Section 3.5, Figure S5 / Figure 7

Record 52: tau1 dependency (windowed PMLG9)  - Section 3.5, Figure 6

Record 72: tau1 dependency (windowless PMLG9)  - Section 3.5, Figure 6

Record 220: tau1 dependency (windowed PMLG5)  - Section 3.5, Figure 6

Record 315-317: Sensitivity inverse CP vs CP- Refocused INEPT - Section 3.5, Figure 8


bAsp-Ala experiments:
===================

Record 309: 2D 15N-1H CP- Refocused INEPT experiment (no 1H homonuclear decoupling) - Section 3.6, Figure 9

Record 310: 2D 15N-1H CP- Refocused INEPT experiment (windowed PMLG5) - Section 3.6, Figure 9

Record 311: 1H 1D CRAMPS - Section 3.6, Figure 9

Record 318-332: tau2 dependency of 15N multiplicity - Section 3.6, Figure 10


Cimetdine experiments:
===================

Record 312: One-pulse 1H 1D - Section 3.6, Figure 9

Record 313: 2D 15N-1H CP- Refocused INEPT experiment (windowed PMLG5)  - Section 3.6, Figure 9

Record 314: 1H spin-echo dephasing time (windowed PMLG5) - Section S5, Figure S6