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Transition from dynamic to static disorder in one-dimensional organic semiconductors
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Troisi, Alessandro and Cheung, David L.. (2009) Transition from dynamic to static disorder in one-dimensional organic semiconductors. Journal of Chemical Physics, Vol.131 (No.1). article no. 014703 . ISSN 0021-9606
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Official URL: http://dx.doi.org/10.1063/1.3167406
Abstract
A generic model Hamiltonian is proposed for the study of the transport in a quasi-one-dimensional semiconductor in the charge transport regime intermediate between dynamic localization and static localization due to structural disorder. This intermediate regime may be appropriate for many organic semiconductors, including polymers, discotic liquid crystals, and DNA. The dynamics of the charge carrier is coupled to classical Langevin oscillators whose spectral density can be adjusted to model experimental systems of interest. In the proposed model, the density of states is constant (at constant temperature) and the transition from dynamic to static disorder is controlled by a single parameter. This paper further clarifies that the density of states may not contain all the information needed to describe the charge transport in some materials.
| Item Type: | Journal Article |
|---|---|
| Subjects: | Q Science > QC Physics Q Science > QD Chemistry |
| Divisions: | Faculty of Science > Chemistry Faculty of Science > Centre for Scientific Computing |
| Library of Congress Subject Headings (LCSH): | Organic semiconductors, Polymers -- Electric properties, One-dimensional conductors |
| Journal or Publication Title: | Journal of Chemical Physics |
| Publisher: | American Institute of Physics |
| ISSN: | 0021-9606 |
| Date: | 7 July 2009 |
| Volume: | Vol.131 |
| Number: | No.1 |
| Number of Pages: | 8 |
| Page Range: | article no. 014703 |
| Identification Number: | 10.1063/1.3167406 |
| Status: | Peer Reviewed |
| Publication Status: | Published |
| Access rights to Published version: | Restricted or Subscription Access |
| Funder: | Engineering and Physical Sciences Research Council (EPSRC) |
| Grant number: | EP/E03375X/1 (EPSRC) |
| URI: | http://wrap.warwick.ac.uk/id/eprint/27644 |
Data sourced from Thomson Reuters' Web of Knowledge
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