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Asymmetric transfer hydrogenation of C=O and C=N bonds by tethered Rh-III catalysts

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Matharu, Daljit S., Martins, Jose E. D. and Wills, Martin (2008) Asymmetric transfer hydrogenation of C=O and C=N bonds by tethered Rh-III catalysts. Chemistry - An Asian Journal, Vol.3 (No.8-9). pp. 1374-1383. doi:10.1002/asia.200800189

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Official URL: http://dx.doi.org/10.1002/asia.200800189

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Abstract

Rh-III catalysts containing a tetramethylcyclopentadienyl group linked by a 'tether' to a tosylated diamine ligand have previously been reported by our group for the asymmetric transfer hydrogenation (ATH) of ketones. The extension of these catalysts to the asymmetric reduction of imines, as well as to more highly functionalized substrates is reported. In some cases, the catalysts give better ee values than other methods for these transformations at lower catalyst loadings. The introduction of a methoxy group into the tethering aryl ring does not negate the performance of the catalyst, thus opening up a route to supported derivatives.

Item Type: Journal Item
Subjects: Q Science > QD Chemistry
Divisions: Faculty of Science > Chemistry
Journal or Publication Title: Chemistry - An Asian Journal
Publisher: Wiley - V C H Verlag GmbH & Co. KGaA
ISSN: 1861-4728
Official Date: 2008
Dates:
DateEvent
2008Published
Volume: Vol.3
Number: No.8-9
Number of Pages: 10
Page Range: pp. 1374-1383
DOI: 10.1002/asia.200800189
Status: Peer Reviewed
Publication Status: Published
Funder: Coordenacao de Aperfeicoamento de Pessoal de Ensinol Superior (CAPES, Brazil)

Data sourced from Thomson Reuters' Web of Knowledge

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