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Growth of p- and n-dopable films from electrochemically generated C-60 cations
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Bruno, Carlo, Marcaccio, Massimo, Paolucci, Demis, Castellarin-Cudia, Carla, Goldoni, Andrea, Streletskii, Alexey V., Drewello, Thomas, Barison, Simona, Venturini, Alessandro, Zerbetto, Francesco and Paolucci, F. (Francesco) (2008) Growth of p- and n-dopable films from electrochemically generated C-60 cations. Journal of the American Chemical Society, Volume 130 (Number 12). pp. 3788-3796. doi:10.1021/ja0733179 ISSN 0002-7863.
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Official URL: http://dx.doi.org/10.1021/ja0733179
Abstract
The formidable electron-acceptor properties Of C-60 contrast with its difficult oxidations. Only recently it has become possible to achieve reversibility of more than one electrochemical anodic process versus the six reversible cathodic reductions. Here we exploit the reactivity of electrochemical oxidations of pure C-60 to grow a film of high thermal and mechanical stability on the anode. The new material differs remarkably from its precursor since it conducts both electrons and holes. Its growth and properties are consistently characterized by a host of techniques that include atomic force microscopy (AFM), Raman and infrared spectroscopies, X-ray-photoelectron spectroscopy (XPS), secondary-ion mass spectrometry (SIMS), scanning electron microscopy and energy-dispersive X-ray analysis (SEM-EDX), matrix-assisted laser desorption/ionization (MALDI), and a variety of electrochemical measurements.
| Item Type: | Journal Article | ||||
|---|---|---|---|---|---|
| Subjects: | Q Science > QD Chemistry | ||||
| Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry | ||||
| Library of Congress Subject Headings (LCSH): | Thin films, Electrochemistry, Cations, Oxidation | ||||
| Journal or Publication Title: | Journal of the American Chemical Society | ||||
| Publisher: | American Chemical Society | ||||
| ISSN: | 0002-7863 | ||||
| Official Date: | 26 March 2008 | ||||
| Dates: |
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| Volume: | Volume 130 | ||||
| Number: | Number 12 | ||||
| Number of Pages: | 9 | ||||
| Page Range: | pp. 3788-3796 | ||||
| DOI: | 10.1021/ja0733179 | ||||
| Status: | Peer Reviewed | ||||
| Publication Status: | Published | ||||
| Access rights to Published version: | Restricted or Subscription Access | ||||
| Funder: | Università di Bologna, Italy. Ministero dell'università e della ricerca scientifica e tecnologica |
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