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Catalytic alkene cyclohydroamination via an imido mechanism
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Gott, Andrew L., Clarke, Adam J., Clarkson, Guy J. and Scott, Peter (2008) Catalytic alkene cyclohydroamination via an imido mechanism. Chemical Communications, Vol.44 (No.12). pp. 1422-1424. doi:10.1039/b718373a ISSN 1359-7345.
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Official URL: http://dx.doi.org/10.1039/b718373a
Abstract
Chiral-at-metal half-sandwich diamide complexes catalyse enantioselective cyclohydroamination of aminoalkenes at unexpectedly high rates given their high coordination number and steric bulk; substantial evidence is presented which argues against the established sigma-bond insertion process and is strongly indicative of an imido [2+2] cycloaddition mechanism.
| Item Type: | Journal Article | ||||
|---|---|---|---|---|---|
| Subjects: | Q Science > QD Chemistry | ||||
| Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry | ||||
| Library of Congress Subject Headings (LCSH): | Alkenes, Amination, Enantioselective catalysis, Catalysts, Zirconium | ||||
| Journal or Publication Title: | Chemical Communications | ||||
| Publisher: | Royal Society of Chemistry | ||||
| ISSN: | 1359-7345 | ||||
| Official Date: | 2008 | ||||
| Dates: |
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| Volume: | Vol.44 | ||||
| Number: | No.12 | ||||
| Number of Pages: | 3 | ||||
| Page Range: | pp. 1422-1424 | ||||
| DOI: | 10.1039/b718373a | ||||
| Status: | Peer Reviewed | ||||
| Publication Status: | Published | ||||
| Access rights to Published version: | Restricted or Subscription Access | ||||
| Funder: | Engineering and Physical Sciences Research Council (EPSRC) |
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