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Dynamics of H-loss in adenine via the (1)pi sigma* state using a combination of ns and fs laser spectroscopy
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Wells, Kym Lewis, Roberts, Gareth M. and Stavros, Vasilios G.. (2007) Dynamics of H-loss in adenine via the (1)pi sigma* state using a combination of ns and fs laser spectroscopy. Chemical Physics Letters, Vol.446 (No.1-3). pp. 20-24. ISSN 0009-2614
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Official URL: http://dx.doi.org/10.1016/j.cplett.2007.08.040
Abstract
One of the key questions underlying adenine's photochemistry following 266 nm excitation is whether or not the dissociative (1)pi sigma* state plays an active role in the ensuing dynamics. This work describes how laser fluence studies on the Ad(+) and H+ following photo-excitation using a combination of ns and fs UY pulses with time-of-flight mass-spectrometry, provides new evidence that implicates the contentious participation of the (1)pi sigma* state in the photochemistry of adenine. (C) 2007 Elsevier B.V. All rights reserved.
| Item Type: | Journal Article |
|---|---|
| Subjects: | Q Science > QD Chemistry |
| Divisions: | Faculty of Science > Chemistry |
| Library of Congress Subject Headings (LCSH): | Photochemistry, Adenine, Laser spectroscopy, Elimination reactions |
| Journal or Publication Title: | Chemical Physics Letters |
| Publisher: | Elsevier BV |
| ISSN: | 0009-2614 |
| Date: | 26 September 2007 |
| Volume: | Vol.446 |
| Number: | No.1-3 |
| Number of Pages: | 5 |
| Page Range: | pp. 20-24 |
| Identification Number: | 10.1016/j.cplett.2007.08.040 |
| Status: | Peer Reviewed |
| Publication Status: | Published |
| Funder: | Engineering and Physical Sciences Research Council (EPSRC), Royal Society (Great Britain) |
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| URI: | http://wrap.warwick.ac.uk/id/eprint/31332 |
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