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Magnetic phases in the Kagome staircase compound Co3V2O8 studied using powder neutron diffraction
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Wilson, N. R., Petrenko, Oleg and Chapon, L. C. (2007) Magnetic phases in the Kagome staircase compound Co3V2O8 studied using powder neutron diffraction. Physical Review B, Vol.75 (No.9). Article: 094432. doi:10.1103/PhysRevB.75.094432 ISSN 1098-0121.
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Official URL: http://dx.doi.org/10.1103/PhysRevB.75.094432
Abstract
The low temperature properties of the Kagome-type system Co3V2O8 have been studied by powder neutron diffraction both in zero field and in applied magnetic fields of up to 8 T. Below 6 K, the zero-field ground state is ferromagnetic with the magnetic moments aligned along the a axis. The size of the moment on one of the two Co sites, the so-called cross-tie site, is considerably reduced compared to the fully polarized state. The application of a magnetic field in this phase is found to rapidly enhance the cross-tie site magnetic moment, which reaches the expected value of similar to 3 mu(B) by the maximum applied field of 8 T. Different reorientation behaviors are found for the Co cross-tie and spine sites, suggesting a more pronounced easy-axis anisotropy for moments on the spine sites. Rietveld refinements reveal that a simple model, where the spins on both cross-tie and spine sites rotate in the ac plane in a magnetic field, reproduces the experimental diffraction patterns well. In addition, it is found that at higher temperatures and moderate magnetic fields, the incommensurate antiferromagnetic order, corresponding to a transverse sinusoidal modulation above 8 K, is suppressed to be replaced by ferromagnetic order.
Item Type: | Journal Article | ||||
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Subjects: | Q Science > QC Physics | ||||
Divisions: | Faculty of Science, Engineering and Medicine > Science > Physics | ||||
Journal or Publication Title: | Physical Review B | ||||
Publisher: | American Physical Society | ||||
ISSN: | 1098-0121 | ||||
Official Date: | March 2007 | ||||
Dates: |
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Volume: | Vol.75 | ||||
Number: | No.9 | ||||
Number of Pages: | 6 | ||||
Page Range: | Article: 094432 | ||||
DOI: | 10.1103/PhysRevB.75.094432 | ||||
Status: | Peer Reviewed | ||||
Publication Status: | Published | ||||
Access rights to Published version: | Restricted or Subscription Access |
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