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An unexpected directing effect in the asymmetric transfer hydrogenation of α,α-Disubstituted ketones

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Soni, Rina, Collinson, John-Michael, Clarkson, Guy J. and Wills, Martin (2011) An unexpected directing effect in the asymmetric transfer hydrogenation of α,α-Disubstituted ketones. Organic Letters, 13 (16). pp. 4304-4307. doi:10.1021/ol201643v

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Official URL: http://dx.doi.org/10.1021/ol201643v

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Abstract

alpha,alpha-Disubstituted ketones containing an aromatic ring or alkene are reduced in high enantiomeric excess using an asymmetric transfer hydrogenation catalyst. The sense of reduction indicates that the unsaturated region of the ketone adopts a position adjacent to the Ru-bound eta(6)-arene ring in the reduction transition state.

Item Type: Journal Article
Subjects: Q Science > QD Chemistry
Divisions: Faculty of Science > Chemistry
Library of Congress Subject Headings (LCSH): Hydrogenation, Carbonyl compounds, Ketones, Reduction (Chemistry), Catalysis
Journal or Publication Title: Organic Letters
Publisher: American Chemical Society
ISSN: 1523-7060
Official Date: 14 July 2011
Dates:
DateEvent
14 July 2011Published
14 July 2011Accepted
17 June 2011Submitted
Volume: 13
Number: 16
Page Range: pp. 4304-4307
DOI: 10.1021/ol201643v
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access

Data sourced from Thomson Reuters' Web of Knowledge

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