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Efficient dynamic nuclear polarization at high magnetic fields
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Morley, Gavin, Tol, J. (Johan) van, Ardavan, Arzhang, Porfyrakis, Kyriakos, Zhang, Jinying and Briggs, Andrew H. (2007) Efficient dynamic nuclear polarization at high magnetic fields. Physical Review Letters, Vol.98 (No.22). pp. 220501-1. doi:10.1103/PhysRevLett.98.220501 ISSN 0031-9007.
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Official URL: http://dx.doi.org/10.1103/PhysRevLett.98.220501
Abstract
By applying a new technique for dynamic nuclear polarization involving simultaneous excitation of electronic and nuclear transitions, we have enhanced the nuclear polarization of the nitrogen nuclei in 15N@C60 by a factor of 103 at a fixed temperature of 3 K and a magnetic field of 8.6 T, more than twice the maximum enhancement reported to date. This methodology will allow the initialization of the nuclear qubit in schemes exploiting N@C60 molecules as components of a quantum information processing device.
| Item Type: | Journal Article | ||||
|---|---|---|---|---|---|
| Subjects: | Q Science > QC Physics | ||||
| Divisions: | Faculty of Science, Engineering and Medicine > Science > Physics | ||||
| Library of Congress Subject Headings (LCSH): | Polarization (Nuclear Physics), Magnetic fields | ||||
| Journal or Publication Title: | Physical Review Letters | ||||
| Publisher: | American Physical Society | ||||
| ISSN: | 0031-9007 | ||||
| Official Date: | 31 May 2007 | ||||
| Dates: |
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| Volume: | Vol.98 | ||||
| Number: | No.22 | ||||
| Number of Pages: | 4 | ||||
| Page Range: | pp. 220501-1 | ||||
| DOI: | 10.1103/PhysRevLett.98.220501 | ||||
| Status: | Peer Reviewed | ||||
| Publication Status: | Published | ||||
| Access rights to Published version: | Restricted or Subscription Access | ||||
| Funder: | Engineering and Physical Sciences Research Council (EPSRC), Quantum Information Processing Interdisciplinary Research Collaboration (QIPIRC), National High Magnetic Field Laboratory (NHMFL), National Science Foundation (U.S.) (NSF), Florida, United States. Dept of Energy | ||||
| Grant number: | GR/S82176/01 (EPSRC), EP/D048559/1 (EPSRC), GR/S15808/01 (EPSRC), GR/S23506 (EPSRC), DMR-0084173 (NSF) | ||||
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