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The spontaneous loss of coherence catastrophe in fourier transform ion cyclotron resonance mass spectrometry

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Aizikov, Konstantin, Mathur, Raman and O’Connor, Peter B. (2009) The spontaneous loss of coherence catastrophe in fourier transform ion cyclotron resonance mass spectrometry. Journal of The American Society for Mass Spectrometry, Vol.20 (No.2). pp. 247-256. doi:10.1016/j.jasms.2008.09.028 ISSN 1044-0305.

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Official URL: http://dx.doi.org/10.1016/j.jasms.2008.09.028

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Abstract

The spontaneous loss of coherence catastrophe (SLCC) is a frequently observed, yet poorly studied, space-charge related effect in Fourier-transform ion cyclotron resonance mass spectrometry (FTICR-MS). This manuscript presents an application of the filter diagonalization method (FDM) in the analysis of this phenomenon. The temporal frequency behavior reproduced by frequency shift analysis using the FDM shows the complex nature of the SLCC, which can be explained by a combination of factors occurring concurrently, governed by electrostatics and ion packet trajectories inside the ICR cell.

Item Type: Journal Article
Subjects: Q Science > QD Chemistry
T Technology > TK Electrical engineering. Electronics Nuclear engineering
Divisions: Faculty of Science, Engineering and Medicine > Science > Chemistry
Library of Congress Subject Headings (LCSH): Fourier transform spectroscopy, Ion cyclotron resonance spectrometry, Mass spectrometry, Space charge
Journal or Publication Title: Journal of The American Society for Mass Spectrometry
Publisher: Springer New York LLC
ISSN: 1044-0305
Official Date: February 2009
Dates:
DateEvent
February 2009Published
Volume: Vol.20
Number: No.2
Number of Pages: 10
Page Range: pp. 247-256
DOI: 10.1016/j.jasms.2008.09.028
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Open Access (Creative Commons)
Funder: National Institutes of Health (U.S.) (NIH), National Center for Research Resources (U.S.) (NCRR), National Heart, Lung, and Blood Institute (NHLBI)
Grant number: P41-RR10888 (NIH/NCRR), NO1 HV28178 (NIH/NHLBI), R01GM078293 (NIH/NHLBI)

Data sourced from Thomson Reuters' Web of Knowledge

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