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Electrochemical mapping reveals direct correlation between heterogeneous electron-transfer kinetics and local density of states in diamond electrodes
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Patten, Hollie V., Meadows, Katherine E., Hutton, Laura A., Iacobini, James G., Battistel, Dario, McKelvey, Kim M. (Kim Martin), Colburn, Alex W., Newton, Mark E., Macpherson, Julie V. and Unwin, Patrick R. (2012) Electrochemical mapping reveals direct correlation between heterogeneous electron-transfer kinetics and local density of states in diamond electrodes. Angewandte Chemie International Edition, Volume 51 (Number 28). pp. 7002-7006. doi:10.1002/anie.201203057 ISSN 1433-7851.
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WRAP_Patten, Angewandte, 2012.pdf - Submitted Version Download (1529Kb) | Preview |
Official URL: http://dx.doi.org/10.1002/anie.201203057
Abstract
Conducting carbon materials: A multi-microscopy approach shows that local heterogeneous electron-transfer rates at conducting diamond electrodes correlate with the local density of electronic states. This model of electroactivity is of considerable value for the rational design of conducting diamond electrochemical technologies, and also provides key general insights on electrode structure controls in electrochemical kinetics
Item Type: | Journal Article | ||||
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Subjects: | Q Science > QD Chemistry | ||||
Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry Faculty of Science, Engineering and Medicine > Research Centres > Molecular Organisation and Assembly in Cells (MOAC) Faculty of Science, Engineering and Medicine > Science > Physics |
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Library of Congress Subject Headings (LCSH): | Electrochemistry, High resolution electron microscopy, Chemical kinetics, Charge exchange, Electrodes | ||||
Journal or Publication Title: | Angewandte Chemie International Edition | ||||
Publisher: | Wiley - V C H Verlag GmbH & Co. KGaA | ||||
ISSN: | 1433-7851 | ||||
Official Date: | July 2012 | ||||
Dates: |
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Volume: | Volume 51 | ||||
Number: | Number 28 | ||||
Page Range: | pp. 7002-7006 | ||||
DOI: | 10.1002/anie.201203057 | ||||
Status: | Peer Reviewed | ||||
Publication Status: | Published | ||||
Access rights to Published version: | Restricted or Subscription Access | ||||
Funder: | Engineering and Physical Sciences Research Council (EPSRC) , University of Warwick. Molecular Organisation and Assembly in Cells, Element Six, European Research Council (ERC), Advantage West Midlands (AWM), European Regional Development Fund (ERDF) | ||||
Grant number: | ERC-2009-AdG 247143-QUANTIF |
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