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Orthogonal modification of norbornene-functional degradable polymers

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Williams, Rebecca J., Barker, Ian A., O’Reilly, Rachel K. and Dove, Andrew P. (2012) Orthogonal modification of norbornene-functional degradable polymers. ACS Macro Letters, Vol.1 (No.11). pp. 1285-1290. doi:10.1021/mz300496q

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Official URL: http://dx.doi.org/10.1021/mz300496q

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Abstract

Well-defined norbornene-functional poly(carbonate)s were prepared by ring-opening polymerization and utilized as multireactive polymeric scaffolds in a range of postpolymerization modifications. The norbornene-functional handles were shown to undergo facile reaction with azides via a 1,3-dipolar cycloaddition, tetrazines in the inverse electron demand Diels–Alder reaction and thiols via radical thiol-ene coupling. Furthermore, the above-mentioned chemistries were demonstrated in a sequential one-pot, three-step modification reaction illustrating the potential of these polymers as scaffolds to access multifunctionalized materials in an undemanding manner.

Item Type: Journal Article
Divisions: Faculty of Science, Engineering and Medicine > Science > Chemistry
Journal or Publication Title: ACS Macro Letters
Publisher: American Chemical Society
ISSN: 2161-1653
Official Date: 2012
Dates:
DateEvent
2012Published
Volume: Vol.1
Number: No.11
Page Range: pp. 1285-1290
DOI: 10.1021/mz300496q
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access

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