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Highly frustrated magnetism in SrHo_{2}O_{4}: coexistence of two types of short-range order
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Young, Olga, Wildes, Andrew R., Manuel, P., Ouladdiaf, B., Khalyavin, D. D., Balakrishnan, Geetha and Petrenko, Oleg (2013) Highly frustrated magnetism in SrHo_{2}O_{4}: coexistence of two types of short-range order. Physical Review B (Condensed Matter and Materials Physics), Volume 88 (Number 2). Article number 024411 . doi:10.1103/PhysRevB.88.024411 ISSN 1098-0121.
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Official URL: http://dx.doi.org/10.1103/PhysRevB.88.024411
Abstract
SrHo2O4 is a geometrically frustrated magnet in which the magnetic Ho3+ ions form honeycomb layers connected through a network of zigzag chains. At low-temperature two distinct types of short-range magnetic order can be inferred from single-crystal diffraction data, collected using both polarized and unpolarized neutrons. In the (hk0) plane the diffuse scattering is most noticeable around the k=0 positions and its intensity rapidly increases at temperatures below 0.7 K. In addition, planes of diffuse scattering at Q=(hk±l/2) are visible at temperatures as high as 4.5 K. These planes coexist with the broad peaks of diffuse scattering in the (hk0) plane at low temperatures. Correlation lengths associated with the broad peaks are L≈150 Å in the a–b plane and L≈190 Å along the c axis, while the correlation length associated with the diffuse scattering planes is L≈230 Å along the c axis at the lowest temperature. Both types of diffuse scattering are elastic in nature. The highly unusual coexistence of the two types of diffuse scattering in SrHo2O4 is likely to be the result of the presence of two crystallographically inequivalent sites for Ho3+ in the unit cell.
Item Type: | Journal Article | ||||
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Divisions: | Faculty of Science, Engineering and Medicine > Science > Physics | ||||
Journal or Publication Title: | Physical Review B (Condensed Matter and Materials Physics) | ||||
Publisher: | American Physical Society | ||||
ISSN: | 1098-0121 | ||||
Official Date: | 1 July 2013 | ||||
Dates: |
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Volume: | Volume 88 | ||||
Number: | Number 2 | ||||
Page Range: | Article number 024411 | ||||
DOI: | 10.1103/PhysRevB.88.024411 | ||||
Status: | Peer Reviewed | ||||
Publication Status: | Published | ||||
Access rights to Published version: | Restricted or Subscription Access |
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