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Highly frustrated magnetism in SrHo_{2}O_{4}: coexistence of two types of short-range order

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Young, Olga, Wildes, Andrew R., Manuel, P., Ouladdiaf, B., Khalyavin, D. D., Balakrishnan, Geetha and Petrenko, Oleg (2013) Highly frustrated magnetism in SrHo_{2}O_{4}: coexistence of two types of short-range order. Physical Review B (Condensed Matter and Materials Physics), Volume 88 (Number 2). Article number 024411 . doi:10.1103/PhysRevB.88.024411

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Official URL: http://dx.doi.org/10.1103/PhysRevB.88.024411

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Abstract

SrHo2O4 is a geometrically frustrated magnet in which the magnetic Ho3+ ions form honeycomb layers connected through a network of zigzag chains. At low-temperature two distinct types of short-range magnetic order can be inferred from single-crystal diffraction data, collected using both polarized and unpolarized neutrons. In the (hk0) plane the diffuse scattering is most noticeable around the k=0 positions and its intensity rapidly increases at temperatures below 0.7 K. In addition, planes of diffuse scattering at Q=(hk±l/2) are visible at temperatures as high as 4.5 K. These planes coexist with the broad peaks of diffuse scattering in the (hk0) plane at low temperatures. Correlation lengths associated with the broad peaks are L≈150 Å in the a–b plane and L≈190 Å along the c axis, while the correlation length associated with the diffuse scattering planes is L≈230 Å along the c axis at the lowest temperature. Both types of diffuse scattering are elastic in nature. The highly unusual coexistence of the two types of diffuse scattering in SrHo2O4 is likely to be the result of the presence of two crystallographically inequivalent sites for Ho3+ in the unit cell.

Item Type: Journal Article
Divisions: Faculty of Science > Physics
Journal or Publication Title: Physical Review B (Condensed Matter and Materials Physics)
Publisher: American Physical Society
ISSN: 1098-0121
Official Date: 1 July 2013
Dates:
DateEvent
1 July 2013Published
Volume: Volume 88
Number: Number 2
Page Range: Article number 024411
DOI: 10.1103/PhysRevB.88.024411
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access

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