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“Magic” surface clustering of borazines driven by repulsive intermolecular forces

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Kervyn, Simon, Kalashnyk, Nataliya, Riello, Massimo, Moreton, Ben, Tasseroul, Jonathan, Wouters, Johan, Jones, T. S. (Tim S.), De Vita, Alessandro, Costantini, Giovanni and Bonifazi, D. (2013) “Magic” surface clustering of borazines driven by repulsive intermolecular forces. Angewandte Chemie International Edition, Volume 52 (Number 29). pp. 7410-7414. doi:10.1002/anie.201300948

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Official URL: http://dx.doi.org/10.1002/anie.201300948

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Abstract

It's a kind of magic: Hydroxy pentaaryl borazine molecules self-assemble into small clusters (see structure) on Cu(111) surfaces, whereas with symmetric hexaaryl borazine molecules large islands are obtained. Simulations indicate that the observed “magic” cluster sizes result from long-range repulsive Coulomb forces arising from the deprotonation of the B[BOND]OH groups of the hydroxy pentaaryl borazine.

Item Type: Journal Article
Subjects: Q Science > QD Chemistry
Divisions: Faculty of Science > Chemistry
Library of Congress Subject Headings (LCSH): Intermolecular forces, Inorganic cyclic compounds, Microclusters
Journal or Publication Title: Angewandte Chemie International Edition
Publisher: Wiley - V C H Verlag GmbH & Co. KGaA
ISSN: 1433-7851
Official Date: 2013
Dates:
DateEvent
2013Published
Volume: Volume 52
Number: Number 29
Page Range: pp. 7410-7414
DOI: 10.1002/anie.201300948
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access
Funder: European Union (EU), Fonds national de la recherche scientifique (Belgium) (FNRS), Belgium. Politique scientifique fédérale, Italy. Ministero dell'istruzione, dell'università e della ricerca (MIUR), Université de Namur, Engineering and Physical Sciences Research Council (EPSRC), Royal Society (Great Britain), University of Warwick

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