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Spectroscopic and computational study of ligand photodissociation from [Ru(dipyrido[3,2-a:2',3'-c]phenazine)(4-aminopyridine)(4)](2+)

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Ruiu, Tiziana, Garino, Claudio, Salassa, Luca, Pizarro, Ana M., Nervi, Carlo, Gobetto, Roberto and Sadler, P. J. (2010) Spectroscopic and computational study of ligand photodissociation from [Ru(dipyrido[3,2-a:2',3'-c]phenazine)(4-aminopyridine)(4)](2+). European Journal of Inorganic Chemistry, Vol.2010 (No.8). pp. 1186-1195. doi:10.1002/ejic.200900990

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Official URL: http://dx.doi.org/10.1002/ejic.200900990

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Abstract

The new complex [Ru(dppz)(4AP)(4)](2+) (1, in which dppz = dipyrido[3,2-a:2',3'-c]phenazine and 4AP = 4-aminopyridine) has been synthesized, characterized and its photophysical and photochemical properties have been studied by combining spectroscopic and computational [DFT and time-dependent (TD) DFT] methods. Upon irradiation in aqueous solution, complex I selectively photoreleases one 4AP ligand and subsequently coordinates a water molecule to form [Ru(dppz)(4AP)(3)(OH2)](2+).

Item Type: Journal Article
Subjects: Q Science > QD Chemistry
Divisions: Faculty of Science, Engineering and Medicine > Science > Chemistry
Library of Congress Subject Headings (LCSH): Photochemistry, Ruthenium, Density functionals, Ligands, Coordination compounds
Journal or Publication Title: European Journal of Inorganic Chemistry
Publisher: Wiley-VCH Verlag GMBH
ISSN: 1434-1948
Official Date: March 2010
Dates:
DateEvent
March 2010Published
Volume: Vol.2010
Number: No.8
Number of Pages: 10
Page Range: pp. 1186-1195
DOI: 10.1002/ejic.200900990
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access
Funder: Piedmont (Italy), Seventh Framework Programme (European Commission) (FP7), Medical Research Council (Great Britain) (MRC), European Regional Development Fund (ERDF), Advantage West Midlands (AWM)
Grant number: 220281 (FP7)

Data sourced from Thomson Reuters' Web of Knowledge

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