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Screening of new solvents for artemisinin extraction process using ab initio methodology
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Lapkin, Alexei, Peters, Martina, Greiner, Lasse, Chemat, Smai, Leonhard, Kai, Liauw, Marcel A. and Leitner, Walter. (2010) Screening of new solvents for artemisinin extraction process using ab initio methodology. Green Chemistry, Vol.12 (No.2). pp. 241-251. ISSN 1463-9262
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Official URL: http://dx.doi.org/10.1039/b922001a
Abstract
The solubility of artemisinin in a range of conventional and novel solvents was evaluated using the COSMO-RS approach, and verified experimentally as well as against literature data. The computational method was improved by calibrating against a limited set of experimental data, enhancing the accuracy of the calculations. The optimised method was shown to be in reasonable agreement with experimental data; however, lack of reliable experimental data is identified as an issue. Several novel solvents perceived as green alternatives to conventional solvents were targeted and shown to offer good solubility of artemisinin. Extraction from Artemisia annua by carbonate solvents was experimentally verified.
| Item Type: | Journal Article | ||||
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| Subjects: | Q Science > QD Chemistry T Technology > TP Chemical technology |
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| Divisions: | Faculty of Science > Engineering | ||||
| Library of Congress Subject Headings (LCSH): | Artemisinin, Extraction (Chemistry), Solvent extraction | ||||
| Journal or Publication Title: | Green Chemistry | ||||
| Publisher: | Royal Society of Chemistry | ||||
| ISSN: | 1463-9262 | ||||
| Official Date: | February 2010 | ||||
| Dates: |
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| Volume: | Vol.12 | ||||
| Number: | No.2 | ||||
| Number of Pages: | 11 | ||||
| Page Range: | pp. 241-251 | ||||
| Identification Number: | 10.1039/b922001a | ||||
| Status: | Peer Reviewed | ||||
| Publication Status: | Published | ||||
| Access rights to Published version: | Restricted or Subscription Access | ||||
| Funder: | Engineering and Physical Sciences Research Council (EPSRC), RWTH Aachen University "Tailor Made Fuels from Biomass" | ||||
| Grant number: | EP/F016182/1 (EPSRC), EXC236 (Aachen) | ||||
| URI: | http://wrap.warwick.ac.uk/id/eprint/6476 |
Data sourced from Thomson Reuters' Web of Knowledge
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