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Electrochemistry of nanoparticles
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Kleijn, Steven E. F., Lai, Stanley Chi Shing, Koper, Marc T. M. and Unwin, Patrick R. (2014) Electrochemistry of nanoparticles. Angewandte Chemie International Edition, Volume 53 (Number 14). pp. 3558-3586. doi:10.1002/anie.201306828 ISSN 1433-7851.
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Official URL: http://dx.doi.org/10.1002/anie.201306828
Abstract
Metal nanoparticles (NPs) find widespread application as a result of their unique physical and chemical properties. NPs have generated considerable interest in catalysis and electrocatalysis, where they provide a high surface area to mass ratio and can be tailored to promote particular reaction pathways. The activity of NPs can be analyzed especially well using electrochemistry, which probes interfacial chemistry directly. In this Review, we discuss key issues related to the electrochemistry of NPs. We highlight model studies that demonstrate exceptional control over the NP shape and size, or mass-transport conditions, which can provide key insights into the behavior of ensembles of NPs. Particular focus is on the challenge of ultimately measuring reactions at individual NPs, and relating the response to their structure, which is leading to imaginative experiments that have an impact on electrochemistry in general as well as broader surface and colloid science.
Item Type: | Journal Article | ||||||||
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Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry | ||||||||
Journal or Publication Title: | Angewandte Chemie International Edition | ||||||||
Publisher: | Wiley - V C H Verlag GmbH & Co. KGaA | ||||||||
ISSN: | 1433-7851 | ||||||||
Official Date: | 1 April 2014 | ||||||||
Dates: |
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Volume: | Volume 53 | ||||||||
Number: | Number 14 | ||||||||
Page Range: | pp. 3558-3586 | ||||||||
DOI: | 10.1002/anie.201306828 | ||||||||
Status: | Peer Reviewed | ||||||||
Publication Status: | Published | ||||||||
Access rights to Published version: | Restricted or Subscription Access |
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