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Racemisation of 1-arylethylamines with shvo-type organoruthenium catalysts

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Taylor, Paul C., Apps, James Frederick Shuan-Liang, Livingston, Andrew, Parrett, Mark R., Pounder, Ryan J. and Turner, Andy (2014) Racemisation of 1-arylethylamines with shvo-type organoruthenium catalysts. Synlett, Volume 25 (Number 10). pp. 1391-1394. doi:10.1055/s-0033-1341228

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Official URL: http://dx.doi.org/10.1055/s-0033-1341228

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Abstract

Variation of the electronic nature of the tetraphenyl­cyclopentadienone ligand in organoruthenium complexes influences their utility for racemisation of model chiral amines. Our study highlights the need to balance reactivity and selectivity in the design of racemisation catalysts. Electron-poor Shvo-type catalysts are, at first sight, more effective for racemisation, but yield more by-product; electron-rich complexes are less proficient at racemisation, but lead to less by-product.

Item Type: Journal Article
Journal or Publication Title: Synlett
Publisher: Georg Thieme Verlag
ISSN: 0936-5214
Official Date: June 2014
Dates:
DateEvent
June 2014Published
Volume: Volume 25
Number: Number 10
Page Range: pp. 1391-1394
DOI: 10.1055/s-0033-1341228
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access

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