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Data for Colossal terahertz magnetoresistance at room temperature in epitaxial La0.7Sr0.3MnO3 nanocomposites and single-phase thin films

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Lloyd-Hughes, James, Mosley, C. D. W., Jones, SPP, Lees, Martin R., Chen, A., Jia, Q. X., Choi, E. M. and MacManus-Driscoll, J. L. (2017) Data for Colossal terahertz magnetoresistance at room temperature in epitaxial La0.7Sr0.3MnO3 nanocomposites and single-phase thin films. [Dataset]

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Data deposit - Lloyd-Hughes Nano Letters 2017.zip - Unspecified Version
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Abstract

Colossal magnetoresistance (CMR) is demonstrated at terahertz (THz) frequencies by using terahertz time-domain magnetospectroscopy to examine vertically-aligned nanocomposites (VANs) and planar thin films of La_0.7Sr_0.3MnO_3. At the Curie temperature (room temperature) the THz conductivity of the VAN was dramatically enhanced by over 2 orders of magnitude under the application of a magnetic field, with a non-Drude THz conductivity that increased with frequency. The dc CMR of the VAN is controlled by extrinsic magnetotransport mechanisms such as spin-polarized tunneling between nano-grains. In contrast, we find that THz CMR is dominated by intrinsic, intragrain transport: the mean free path was smaller than the nanocolumn size, and the planar thin-film exhibited similar THz CMR to the VAN. Surprisingly, the observed colossal THz magnetoresistance suggests that the magnetoresistance can be large for ac motion on nanometre length scales, even when the magnetoresistance is negligible on the macroscopic length scales probed by dc transport. This suggests that colossal magnetoresistance at THz frequencies may find use in nanoelectronics and in THz optical components controlled by magnetic fields. The VAN can be scaled in thickness while retaining a high structural quality, and offers a larger THz CMR at room temperature than the planar film.

Item Type: Dataset
Subjects: Q Science > QC Physics
Divisions: Faculty of Science, Engineering and Medicine > Science > Physics
Type of Data: Plain text
Library of Congress Subject Headings (LCSH): Magnetoresistance, Terahertz spectroscopy, Nanocomposites (Materials), Thin films
Publisher: University of Warwick, Department of Physics
Official Date: 16 March 2017
Dates:
DateEvent
16 March 2017Published
14 March 2017Accepted
Status: Not Peer Reviewed
Publication Status: Published
Media of Output (format): .txt
Access rights to Published version: Open Access (Creative Commons)
Copyright Holders: University of Warwick
Description:

figure1(c)-FC
figure1(c)-FC-magnetisation-v-temperature
figure1(c)-ZFC
figure1(c)-ZFC, figure1(c)-ZFC-magnetisation-v-temperature
figure2(a)-sigma1-v-frequency
figure2(b)-dc-rho(10K)-rho(T)-v-temperature
figure2(b)-sigma0-v-temperature
figure3-(a)-VAN-sigma1-v-freq-at-B=0T-and-B=4T-T50K
figure3-(b)-VAN-sigma1-v-freq-at-B=0T-T200K
figure3-(b)-VAN-sigma1-v-freq-at-B=2T-T200K
figure3-(b)-VAN-sigma1-v-freq-at-B=4T-T200K
figure3-(b)-VAN-sigma1-v-freq-at-B=6T-T200K
figure3-(b)-VAN-sigma1-v-freq-at-B=6T-T200K
figure3-(b)-VAN-sigma1-v-freq-at-B=6T-T200K
figure3-(c)-VAN-sigma1-v-freq-at-B=2T-T300K
figure3-(c)-VAN-sigma1-v-freq-at-B=4T-T300K
figure3-(c)-VAN-sigma1-v-freq-at-B=6T-T300K
figure3-(c)-VAN-sigma1-v-freq-at-B=8T-T300K
figure3-(d)-LSMO-sigma1-v-freq-at-B=0T-T300K
figure3-(d)-LSMO-sigma1-v-freq-at-B=2T-T300K
figure3-(d)-LSMO-sigma1-v-freq-at-B=4T-T300K
figure3-(d)-LSMO-sigma1-v-freq-at-B=6T-T300K
figure3-(d)-LSMO-sigma1-v-freq-at-B=8T-T300K

RIOXX Funder/Project Grant:
Project/Grant IDRIOXX Funder NameFunder ID
EP/H003444/2[EPSRC] Engineering and Physical Sciences Research Councilhttp://dx.doi.org/10.13039/501100000266
UNSPECIFIEDNational Aeronautics and Space Administrationhttp://dx.doi.org/10.13039/100000104
UNSPECIFIEDOffice of Sciencehttp://dx.doi.org/10.13039/100006132
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