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Spontaneous emulsification as a function of material exchange.
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Spooner, Stephen, Li, Zushu and Sridhar, Seetharaman (2017) Spontaneous emulsification as a function of material exchange. Scientific Reports, 7 (1). 5450. doi:10.1038/s41598-017-05861-5
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Official URL: http://doi.org/10.1038/s41598-017-05861-5
Abstract
Direct visualization at 1873 K of 0% to 8% molten FeAl droplets suspended in a SiO2 enriched oxide medium was carried out to image the evolution of droplet morphology during reaction between Al and SiO2. Phenomena such as perturbation growth, necking and budding of offspring droplets from a bulk body are observed. The observations are used to discuss and inform a new approach to the nature of interfacial tension and the impact this has on concepts used to define interfacial tension for a two phase system with material exchange across the interface. The mapping of global interfacial tension coupled with free energy dissipation has been used to give an energetic reasoning as to the behaviour seen with respect to aluminium content in the metal phase.
| Item Type: | Journal Article | ||||||
|---|---|---|---|---|---|---|---|
| Subjects: | T Technology > TA Engineering (General). Civil engineering (General) | ||||||
| Divisions: | Faculty of Science > WMG (Formerly the Warwick Manufacturing Group) | ||||||
| SWORD Depositor: | Library Publications Router | ||||||
| Library of Congress Subject Headings (LCSH): | Lightweight materials -- Industrial applications, Surface tension, Steel-aluminum alloys, Iron-aluminum alloys, Silicon compounds | ||||||
| Journal or Publication Title: | Scientific Reports | ||||||
| Publisher: | Nature Publishing Group | ||||||
| ISSN: | 2045-2322 | ||||||
| Official Date: | 14 July 2017 | ||||||
| Dates: |
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| Date of first compliant deposit: | 3 August 2017 | ||||||
| Volume: | 7 | ||||||
| Number: | 1 | ||||||
| Number of Pages: | 12 | ||||||
| Article Number: | 5450 | ||||||
| DOI: | 10.1038/s41598-017-05861-5 | ||||||
| Status: | Peer Reviewed | ||||||
| Publication Status: | Published | ||||||
| Publisher Statement: | ** From PubMed via Jisc Publications Router. ** History: ** received: 17-01-2017 ** accepted: 05-06-2017 | ||||||
| Access rights to Published version: | Open Access | ||||||
| Funder: | Tata Steel, Engineering and Physical Sciences Research Council (EPSRC) | ||||||
| Grant number: | 1356074 (EPSRC) |
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