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Thiol-reactive (co)polymer scaffolds comprising organic arsenical acrylamides

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Footman, Charlotte, de Jongh, Patrick A. J. M., Tanaka, Joji, Peltier, Raoul, Kempe, Kristian, Davis, Thomas P. and Wilson, Paul (2017) Thiol-reactive (co)polymer scaffolds comprising organic arsenical acrylamides. Chemical Communications, 53 (60). pp. 8447-8450. doi:10.1039/c7cc03880a

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Official URL: http://dx.doi.org/10.1039/c7cc03880a

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Abstract

Novel, well-defined organic arsenical homopolymers (Đ = 1.10–1.40) have been synthesised via RAFT polymerisation. Copolymerisation of the As-functional monomer with dimethylacrylamide yielded non-toxic polymer scaffolds (Đ ≈ 1.10) that could be manipulated in response to pH and undergo sequential reduction and substitution in the presence of thiols including cysteine and glutathione.

Item Type: Journal Article
Subjects: Q Science > QD Chemistry
Divisions: Faculty of Science > Chemistry
Library of Congress Subject Headings (LCSH): Polymerization, Polymers, Block copolymers, Thiols, Arsenic compounds
Journal or Publication Title: Chemical Communications
Publisher: Royal Society of Chemistry
ISSN: 1359-7345
Official Date: 6 July 2017
Dates:
DateEvent
6 July 2017Available
6 July 2017Accepted
Date of first compliant deposit: 8 September 2017
Volume: 53
Number: 60
Page Range: pp. 8447-8450
DOI: 10.1039/c7cc03880a
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access
RIOXX Funder/Project Grant:
Project/Grant IDRIOXX Funder NameFunder ID
UNSPECIFIEDMonash-Warwick AllianceUNSPECIFIED
CE140100036[ARC] Australian Research Councilhttp://dx.doi.org/10.13039/501100000923
EP/F500378/1, MOAC-DTC [EPSRC] Engineering and Physical Sciences Research Councilhttp://dx.doi.org/10.13039/501100000266
APP1109945National Health and Medical Research Councilhttp://dx.doi.org/10.13039/501100000925
APP1109945[ARC] Australian Research Councilhttp://dx.doi.org/10.13039/501100000923
Australian Laureate Fellowship[ARC] Australian Research Councilhttp://dx.doi.org/10.13039/501100000923
ECF/2015-075 Leverhulme Trusthttp://dx.doi.org/10.13039/501100000275
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