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Reaction pathways involved in CH4 conversion on Pd/Al2O3 catalysts : TAP as a powerful tool for the elucidation of the effective role of the metal/support interface
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Renème, Y., Pietrzyk, S., Dhainaut, F., Chaar, M., van Veen, André C. and Granger, Pascal (2016) Reaction pathways involved in CH4 conversion on Pd/Al2O3 catalysts : TAP as a powerful tool for the elucidation of the effective role of the metal/support interface. Frontiers in Chemistry, 4 . 7. doi:10.3389/fchem.2016.00007 ISSN 2296-2646.
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WRAP-reaction-pathways-involved-CH4-conversion-van-Veen-2016.pdf - Published Version - Requires a PDF viewer. Available under License Creative Commons Attribution 4.0. Download (3438Kb) | Preview |
Official URL: http://dx.doi.org/10.3389/fchem.2016.00007
Abstract
Temporal Analysis of Products (TAP) investigation on Natural Gas-fueled Vehicle (NGV) catalysts provides information related to the nature of reaction steps involved over noble metals and at the metal-support interface. The determination of accurate kinetic parameters for methane adsorption from single pulse experiments and subsequent investigation of sequential surface reactions from alternative CH4/O2 pulse experiments is the first step toward the establishment of relevant structure/activity relationships which can highlight the importance of the metal/support interface on freshly-prepared and aged single palladium based catalysts.
| Item Type: | Journal Article | ||||||
|---|---|---|---|---|---|---|---|
| Subjects: | T Technology > TP Chemical technology | ||||||
| Divisions: | Faculty of Science, Engineering and Medicine > Engineering > Engineering | ||||||
| Library of Congress Subject Headings (LCSH): | Palladium catalysts , Gas as fuel | ||||||
| Journal or Publication Title: | Frontiers in Chemistry | ||||||
| Publisher: | Frontiers Research Foundation | ||||||
| ISSN: | 2296-2646 | ||||||
| Official Date: | 16 February 2016 | ||||||
| Dates: |
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| Volume: | 4 | ||||||
| Article Number: | 7 | ||||||
| DOI: | 10.3389/fchem.2016.00007 | ||||||
| Status: | Peer Reviewed | ||||||
| Publication Status: | Published | ||||||
| Access rights to Published version: | Open Access (Creative Commons) | ||||||
| Date of first compliant deposit: | 20 October 2017 | ||||||
| Date of first compliant Open Access: | 20 October 2017 | ||||||
| Funder: | France. Agence de l'environnement et de la maîtrise de l'énergie, France. Institut de Recherche en Environnement Industriel (IRENI), France. Agence nationale de la recherche (ANR) |
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