UNSPECIFIED (2003) Magnetic and structural characterisation of the layered materials AMnFe(C2S2O2)(3). In: 8th International Conference on Molecule-Based Magnets (ICMM 2002), OCT 05-10, 2002, VALENCIA, SPAIN.

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Abstract

We present structural and magnetic data on the series of compounds AMn(II)Fe(III)(C2S2O2)(3) with A = N(CnH2n+1)(4) (n = 3-5) or P(C6H5)(4). The tetra-alkyl ammonium compounds are all ferromagnets with T-C = 10 K, whilst the tetraphenyl phosphonium compound is a ferrimagnet with T-N = 15 K. EXAFS spectroscopy shows that there is significant disorder in the orientation of the dithio-oxalate moiety, while high resolution X-ray powder diffraction measurements prove that the dithio-oxalate materials are structurally analogous to the layered oxalates. (C) 2003 Elsevier Science Ltd. All rights reserved.

Item Type:	Conference Item (UNSPECIFIED)
Subjects:	Q Science > QD Chemistry
Journal or Publication Title:	POLYHEDRON
Publisher:	PERGAMON-ELSEVIER SCIENCE LTD
ISSN:	0277-5387
Date:	15 July 2003
Volume:	22
Number:	14-17
Number of Pages:	8
Page Range:	pp. 2317-2324
Publication Status:	Published
Title of Event:	8th International Conference on Molecule-Based Magnets (ICMM 2002)
Location of Event:	VALENCIA, SPAIN
Date(s) of Event:	OCT 05-10, 2002
URI:	http://wrap.warwick.ac.uk/id/eprint/9452

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