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Heteronuclear Ir(III)–Ln(III) luminescent complexes : small-molecule probes for dual modal imaging and oxygen sensing
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Jana, Atanu, Crowston, Bethany J., Shewring, Jonathan R., McKenzie, Luke K., Bryant, Helen E., Botchway, Stanley W., Ward, Andrew D., Amoroso, Angelo J., Baggaley, Elizabeth and Ward, Michael D. (2016) Heteronuclear Ir(III)–Ln(III) luminescent complexes : small-molecule probes for dual modal imaging and oxygen sensing. Inorganic Chemistry, 55 (11). pp. 5623-5633. doi:10.1021/acs.inorgchem.6b00702 ISSN 0020-1669.
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Official URL: http://dx.doi.org/10.1021/acs.inorgchem.6b00702
Abstract
Dinuclear (Ir·Ln) and trinuclear (Ir·Ln2) d−f complexes are investigated for cellular imaging. A range of photophysical, spectroscopic, and imaging-based properties are reported, including relaxivity arising from Gd(III) units and the occurrence of Ir(III) → Eu(III) photoinduced energy-transfer. Noninvasive O2 sensing with Ir·Gd (a potential dual probe: MRI + luminescence) is demonstrated in aqueous solution, full cell media and in vitro, via lifetime mapping and two-photon, phosphorescence lifetime imaging microscopy (PLIM).
Item Type: | Journal Article | ||||
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Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry | ||||
Journal or Publication Title: | Inorganic Chemistry | ||||
Publisher: | American Chemical Society | ||||
ISSN: | 0020-1669 | ||||
Official Date: | 24 May 2016 | ||||
Dates: |
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Volume: | 55 | ||||
Number: | 11 | ||||
Page Range: | pp. 5623-5633 | ||||
DOI: | 10.1021/acs.inorgchem.6b00702 | ||||
Status: | Peer Reviewed | ||||
Publication Status: | Published | ||||
Access rights to Published version: | Restricted or Subscription Access |
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