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Fundamental limits of pulsed quantum light spectroscopy : dipole moment estimation
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Albarelli, Francesco, Bisketzi, Evangelia, Khan, Aiman and Datta, Animesh (2023) Fundamental limits of pulsed quantum light spectroscopy : dipole moment estimation. Physical Review A, 107 (6). 062601 . doi:10.1103/PhysRevA.107.062601 ISSN 1050-2947.
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Official URL: http://doi.org/10.1103/PhysRevA.107.062601
Abstract
We study the fundamental limits of the precision of estimating parameters of a quantum matter system when it is probed by a traveling pulse of quantum light. In particular, we focus on the estimation of the interaction strength between the pulse and a two-level atom, equivalent to the estimation of the dipole moment. Our analysis of single-photon pulses highlights the interplay between the information gained from the absorption of the photon by the atom as measured in absorption spectroscopy and the perturbation to the temporal mode of the photon due to spontaneous emission. Beyond the single-photon regime, we introduce an approximate model to study more general states of light in the limit of short pulses, where spontaneous emission can be neglected. We also show that for a vast class of entangled biphoton states, quantum entanglement between the signal mode interacting with the atom and the idler mode provides no fundamental advantage and the same precision can be obtained with a separable state. We conclude by studying the estimation of the electric dipole moment of a sodium atom using quantum light. Our work initiates a quantum information-theoretic methodology for developing the theory and practice of quantum light spectroscopy.
Item Type: | Journal Article | ||||||||||||
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Subjects: | Q Science > QC Physics | ||||||||||||
Divisions: | Faculty of Science, Engineering and Medicine > Science > Physics | ||||||||||||
Library of Congress Subject Headings (LCSH): | Light -- Scattering, Polarization spectroscopy, Quantum measure theory, Quantum optics, Photons | ||||||||||||
Journal or Publication Title: | Physical Review A | ||||||||||||
Publisher: | American Physical Society | ||||||||||||
ISSN: | 1050-2947 | ||||||||||||
Official Date: | 1 June 2023 | ||||||||||||
Dates: |
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Volume: | 107 | ||||||||||||
Number: | 6 | ||||||||||||
Article Number: | 062601 | ||||||||||||
DOI: | 10.1103/PhysRevA.107.062601 | ||||||||||||
Status: | Peer Reviewed | ||||||||||||
Publication Status: | Published | ||||||||||||
Access rights to Published version: | Restricted or Subscription Access | ||||||||||||
Copyright Holders: | ©2023 American Physical Society | ||||||||||||
Date of first compliant deposit: | 5 June 2023 | ||||||||||||
Date of first compliant Open Access: | 5 June 2023 | ||||||||||||
RIOXX Funder/Project Grant: |
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