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Sequence-controlled multi-block glycopolymers via cu(0) mediated living radical polymerization
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Zhang, Qiang, Collins, Jennifer, Anastasaki, Athina, Wallis, Russell, Mitchell, Daniel A., Becer, C. Remzi, Wilson, Paul and Haddleton, David M. (2014) Sequence-controlled multi-block glycopolymers via cu(0) mediated living radical polymerization. In: Lutz, Jean-Francois, (ed.) Sequence-controlled polymers : synthesis, self-assembly, and properties. ACS Symposium Series, 1170 (1170). Washington DC: American Chemical Society, pp. 327-348. ISBN 9780841230019 (hbk.)
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Official URL: http://pubs.acs.org/doi/abs/10.1021/bk-2014-1170.c...
Abstract
Synthetic glycopolymers with pendant saccharides bind to mammalian carbohydrate-recognition proteins with high affinity due to their multivalency and primary structure. However, glycoproteins function in nature via an exquisitely tuned "glycocode" and mimicking this code remains an interesting challenge in polymer chemistry. In order to address this we have synthesized glycomonomers via a [3+2] cycloaddition reaction between sugar-alkyne and azido-acrylates and these monomers were used to synthesize a series of sequence controlled glycopolymers (SCGP) using single electron transfer living radical polymerization (SET-LRP).
| Item Type: | Book Item | ||||
|---|---|---|---|---|---|
| Divisions: | Faculty of Science, Engineering and Medicine > Science > Chemistry | ||||
| Series Name: | ACS Symposium Series | ||||
| Publisher: | American Chemical Society | ||||
| Place of Publication: | Washington DC | ||||
| ISBN: | 9780841230019 (hbk.) | ||||
| Book Title: | Sequence-controlled polymers : synthesis, self-assembly, and properties | ||||
| Editor: | Lutz, Jean-Francois | ||||
| Official Date: | 2014 | ||||
| Dates: |
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| Volume: | 1170 | ||||
| Number: | 1170 | ||||
| Number of Pages: | 408 | ||||
| Page Range: | pp. 327-348 | ||||
| Status: | Not Peer Reviewed | ||||
| Publication Status: | Published | ||||
| Access rights to Published version: | Restricted or Subscription Access | ||||
| Description: | Article 22 |
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| Conference Paper Type: | Paper | ||||
| Title of Event: | 246th American-Chemical-Society National Meeting | ||||
| Type of Event: | Conference | ||||
| Location of Event: | Indianapolis | ||||
| Date(s) of Event: | 13 Apr 2014 | ||||
| Related URLs: |
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