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Sequence-controlled multi-block glycopolymers via cu(0) mediated living radical polymerization

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Zhang, Qiang, Collins, Jennifer, Anastasaki, Athina, Wallis, Russell, Mitchell, Daniel A., Becer, C. Remzi, Wilson, Paul and Haddleton, David M. (2014) Sequence-controlled multi-block glycopolymers via cu(0) mediated living radical polymerization. In: Lutz, Jean-Francois, (ed.) Sequence-controlled polymers : synthesis, self-assembly, and properties. ACS Symposium Series, 1170 (1170). Washington DC: American Chemical Society, pp. 327-348. ISBN 9780841230019 (hbk.)

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Official URL: http://pubs.acs.org/doi/abs/10.1021/bk-2014-1170.c...

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Abstract

Synthetic glycopolymers with pendant saccharides bind to mammalian carbohydrate-recognition proteins with high affinity due to their multivalency and primary structure. However, glycoproteins function in nature via an exquisitely tuned "glycocode" and mimicking this code remains an interesting challenge in polymer chemistry. In order to address this we have synthesized glycomonomers via a [3+2] cycloaddition reaction between sugar-alkyne and azido-acrylates and these monomers were used to synthesize a series of sequence controlled glycopolymers (SCGP) using single electron transfer living radical polymerization (SET-LRP).

Item Type: Book Item
Divisions: Faculty of Science, Engineering and Medicine > Science > Chemistry
Series Name: ACS Symposium Series
Publisher: American Chemical Society
Place of Publication: Washington DC
ISBN: 9780841230019 (hbk.)
Book Title: Sequence-controlled polymers : synthesis, self-assembly, and properties
Editor: Lutz, Jean-Francois
Official Date: 2014
Dates:
DateEvent
2014Published
Volume: 1170
Number: 1170
Number of Pages: 408
Page Range: pp. 327-348
Status: Not Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access
Description:

Article 22

Conference Paper Type: Paper
Title of Event: 246th American-Chemical-Society National Meeting
Type of Event: Conference
Location of Event: Indianapolis
Date(s) of Event: 13 Apr 2014
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