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Structured catalysts for biofuels transformation into syngas with active components based on perovskite and spinel oxides supported on Mg-doped alumina

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Sadykov, Vladislav, Pavlova, Svetlana, Smal, Ekaterina, Arapova, Marina, Simonov, Mikhail, Mezentseva, Natalia, Rogov, Vladimir, Glazneva, Tatiana, Lukashevich, Anton, Roger, Anne-Cecile, Parkhomenko, Ksenia, van Veen, André C. and Smorygo, Oleg (2017) Structured catalysts for biofuels transformation into syngas with active components based on perovskite and spinel oxides supported on Mg-doped alumina. Catalysis Today, 293-294 . pp. 176-185. doi:10.1016/j.cattod.2017.05.055 ISSN 0920-5861.

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Official URL: http://dx.doi.org/10.1016/j.cattod.2017.05.055

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Abstract

For structured catalysts of biofuels transformation into syngas inexpensive and stable to sintering active components based upon Mg-doped γ-alumina with supported LaNi0.9Ru0.1O3 perovskite or MnCr2O4 spinel promoted by Ru + Ni were developed. Characterization of the surface features, reactivity, catalytic activity and routes of ethanol transformation on these catalysts demonstrated that suppression of support acidity, strong interaction of Ru-Ni alloy nanoparticles with manganese chromite layers on support and a high redox ability provide a high yield of syngas and stability to coking. The most promising active component (2 wt% Ni + 2 wt% Ru)/MnCr2O4/10 wt% MgO − γ-Al2O3 supported on microchannel heat-conducting CrAlO cermet plates demonstrated a high performance and stability to coking in the autothermal reforming of such reactive fuels as glycerol, anisol and turpentine oil.

Item Type: Journal Article
Divisions: Faculty of Science, Engineering and Medicine > Engineering > Engineering
Journal or Publication Title: Catalysis Today
Publisher: Elsevier BV
ISSN: 0920-5861
Official Date: 15 September 2017
Dates:
DateEvent
15 September 2017Published
31 May 2017Available
13 May 2017Accepted
Volume: 293-294
Page Range: pp. 176-185
DOI: 10.1016/j.cattod.2017.05.055
Status: Peer Reviewed
Publication Status: Published
Access rights to Published version: Restricted or Subscription Access
Funder: Commission of the European Communities, Ministry of Education and Science of the Russian Federation

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